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wedrifid comments on Coffee: When it helps, when it hurts - Less Wrong
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Tea has other alkaloids beyond caffeine. Probably the most notable is theanine, which is relaxing. http://en.wikipedia.org/wiki/Theanine
Wonderful stuff, theanine. I converted to green tea extract as my preferred caffeine source once I learned green tea is a good source. (Then I bought bulk theanine powder and explicitly chose my dose!)