Paul Almond's site has many philosophically deep articles on theoretical rationality along LessWrongish assumptions, including but not limited to some great atheology, an attempt to solve the problem of arbitrary UTM choice, a possible anthropic explanation why space is 3D, a thorough defense of Occam's Razor, a lot of AI theory that I haven't tried to understand, and an attempt to explain what it means for minds to be implemented (related in approach to this and this).
Just the list of topics has me drooling ... hope it's worth the read.