Desrtopa comments on Harry Potter and the Methods of Rationality discussion thread, part 28, chapter 99-101 - Less Wrong Discussion
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Maybe even a captive imp is too well concealed to Imperius, although if they're that well cloaked it raises the question of how people even know they exist.
In the original canon, Crouch Jr. as Moody was able to Imperius a spider, which implies that it does not require that the recipient have human language capacity, or even be intelligent.
Also, in canon, in book 7 the protagonists themselves use the Imperius themselves (as part of the break-in to Gringotts.) There we get the best look at the actual mechanics of the Imperius, including that we see Imperius commands being issued telepathically as it were, from the caster's thoughts.