If by "rationalist", the LW community means someone who believes it is possible and desirable to make at least the most important judgements solely by the use of reason operating on empirically demonstrable facts, then I am an ex-rationalist. My "intellectual stew" had simmered into it several forms of formal logic, applied math, and seasoned with a BS in Computer Science at age 23.
By age 28 or so, I concluded that most of the really important things in life were not amenable to this approach, and that the type of thinking I had learned was useful for earning a living, but was woefully inadequate for other purposes.
At age 50, I am still refining the way I think. I come to LW to lurk, learn, and (occasionally) quibble.
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Apologies for coming to this party a bit late. Particularly as I find my own answer really, really frustrating. While I wouldn't say it was an origin per se, getting into reading Overcoming Bias daily a few years back was what crystallised it for me. I'd find myself constantly somewhere between "well, yeah, of course" and "ohhhhhhhhhhhhhhh!" Guess the human brain doesn't tend to do Damascene revelations. We need overwhelming evidence, over a long period of time, to even begin chipping away at our craziest beliefs, and even then it's a step-by-step process.
The analogy I sometimes go over is something most people find fairly obvious like egalitarianism. You don't find many people who would attest to being pro-inequality. But all the same, you find very few people who have genuinely thought through what it means to be in favour of equality and really try to fit that into everyday life. The first step to becoming a rationalist is to admit how irrational everyone is without monumental efforts to the contrary.
BTW, I am totally on the road to de-Catholicising my mother. This is on the order of converting Dubya to Islam, so if I can manage that I'm awarding myself an honorary brown belt.
WRT to de-Catholicising your mother: it has been rightly said that Catholicism is the most rational and consistent of all the religions. So, it would be a pity if you dissuaded her from Catholicism and inadvertently landed her in a less rational religion!