In an Open Thread comment beriukay mentioned that he's reading C.S. Lewis' Mere Christianity. I've been reading it too, for interesting reasons.
In my case it so happened that I started discussing faith with a long-time online friend whose spiritual views I didn't yet know, and he turned out to be a Christian with a high regard for the Bible, who also has an interest in science. As our discussion turned to our readings on spirituality, I acknowledged (I think it was me) that I probably spent more time on books that reinforce my point of view than on books that challenge it, perhaps a case of confirmation bias. (I've been exposed to many poor arguments for Christianity, and dismissed them; but possibly that was largely a function of having started out with that bottom line already written and picking arguments I wouldn't have much trouble refuting.)
In the spirit of experiment we agreed to a "trade" - he would read (thoughtfully and with an open mind) a book of my choosing on reasons to doubt faith, and I'd do the same with a book he chose on Christianity.
So the idea here is to pick a book that's the "best argument from the other side" (as in quote 3 here).
I recommended The God Delusion - I'm not sure if that's the best choice given the above intent, but it's what came to mind on the spot.
Would you make a different choice? If so, what?
Yeah. Then again that was probably "best" in the same sense that TGD was "best" for me: what came to mind on the spot. He's probably read a bunch of other books (and obviously, the Bible), MC was his answer to "which work is most likely to get an open-minded atheist to take one step in my direction".
In fact there were plenty of things in Mere Christianity that I agreed with, it just didn't make much of an impression on me as an argument for the existence of God. It boils down to "we have a strong intuition that there is an objective morality, therefore God".
(ETA: now that I think of it, though, he may have recommended the book also as an answer to the question "what is it exactly that you believe in". Looking back, there may have been some ambiguity to our agreement.)