Things that require nothing, just you. At least in the short term. (e.g., it’s ok to think about what question would be worthwhile to ask on Lesswrong.) I myself sometimes have specific questions from my studies and/or practical matters, which are excellent for this purpose. But the supply of these questions usually is much less than the time I have for pondering them.
I tend to favor your own approach - think about whatever I'm working on. The solution to not having enough questions is to always keep a question around which is A: hard enough that you're unlikely to solve it during a brief wait, and B: in a state where you can work on it without something to write on. Combining these two is not always easy, so you sometimes need to plan ahead.
Departing a bit from the question as stated, adding a phone(and headphones), I've also found that listening to audiobooks is a good way to use e.g. a commute.