Dominic Cummings, a strategist who worked on Brexit. He is surprisingly rationalist-aligned and has very interesting thoughts at his blog.
Drew Endy's a professor at Stanford and synthetic biology pioneer. I discovered him via this talk he gave at a hacker conference about programming DNA. He unfortunately doesn't have a ton of recent public content, but I recommend watching that talk I linked and reading this interview. Two of my favorite quotes of his are (from memory so paraphrased), "biology is nanotech that works" and "what's the most advanced thing on a person's desk. It's not their iPhone; it's the plant they keep there."
I think Drew (also) satisfies most of your desiderata.
David Ha's (Twitter, blog) one of the more interesting deep learning researchers I follow. He works loosely on Model-based Reinforcement Learning and Evolutionary Algorithms, but in practice seems to explore whatever interests him. His most recent paper, Weight Agnostic Neural Networks looks at what happens when you do architecture search over neural nets initialized with random weights to try and better understand how much work structure is doing in neural nets.
I believe David satisfies all of your desiderata.
I'm not sure if he's an unusual thinker by the standards of people on LessWrong, but I really like journalist Richard Meadow and his writing on The Deep Dish blog - https://thedeepdish.org. He does a good job of making a lot of the topics that are discussed in this forum (and other areas, including finance and optionality) accessible and fun to read.
I'd characterise him as an unusual thinker by the standards of the general population, and very good at packaging these unusual ideas in a palatable way for the general population.
Some (optional!) desiderata to guide your recommendation:
Feel free to disregard these criteria if it doesn't work for answering the question! :)